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Pauline Jacquet David Daudé Janek Bzdrenga Patrick Masson Mikael Elias Eric Chabrière 《Environmental science and pollution research international》2016,23(9):8200-8218
Organophosphorus chemicals are highly toxic molecules mainly used as pesticides. Some of them are banned warfare nerve agents. These compounds are covalent inhibitors of acetylcholinesterase, a key enzyme in central and peripheral nervous systems. Numerous approaches, including chemical, physical, and biological decontamination, have been considered for developing decontamination methods against organophosphates (OPs). This work is an overview of both validated and emerging strategies for the protection against OP pollution with special attention to the use of decontaminating enzymes. Considerable efforts have been dedicated during the past decades to the development of efficient OP degrading biocatalysts. Among these, the promising biocatalyst SsoPox isolated from the archaeon Sulfolobus solfataricus is emphasized in the light of recently published results. This hyperthermostable enzyme appears to be particularly attractive for external decontamination purposes with regard to both its catalytic and stability properties. 相似文献
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Sari Kontunen-Soppela Juha Parviainen Mikael Brosché Ramesh C. Thakur Jaakko Kangasjärvi David F. Karnosky 《Environmental pollution (Barking, Essex : 1987)》2010,158(4):959-968
Gene expression responses of paper birch (Betula papyrifera) leaves to elevated concentrations of CO2 and O3 were studied with microarray analyses from three time points during the summer of 2004 at Aspen FACE. Microarray data were analyzed with clustering techniques, self-organizing maps, K-means clustering and Sammon's mappings, to detect similar gene expression patterns within sampling times and treatments. Most of the alterations in gene expression were caused by O3, alone or in combination with CO2. O3 induced defensive reactions to oxidative stress and earlier leaf senescence, seen as decreased expression of photosynthesis- and carbon fixation-related genes, and increased expression of senescence-associated genes. The effects of elevated CO2 reflected surplus of carbon that was directed to synthesis of secondary compounds. The combined CO2 + O3 treatment resulted in differential gene expression than with individual gas treatments or in changes similar to O3 treatment, indicating that CO2 cannot totally alleviate the harmful effects of O3. 相似文献
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Mikael van Deurs Jane W. Behrens Thomas Warnar John Fleng Steffensen 《Marine Biology》2011,158(8):1781-1789
The commercially and ecologically valuable sandeel (Ammodytes ssp.) make distinct vertical shifts between an inactive stage,
during which they seek refuge in the sand, and a pelagic schooling stage, during which they forage. This characteristic discontinuous
foraging pattern constitutes a challenge to fishery biologists and has consequences for a wide range of predators ranging
from birds and mammals to commercially important species. However, experimental studies that shed light on the primary drivers
of foraging activity in fish are rare. In the present study, whole schools of sandeel (A. tobianus) were caught in August in east Denmark (65°02′30N; 12°37′00E) and kept in large tanks in the laboratory. It was found that
the amount of food ingested and memory of past days feeding history are primary drivers of foraging activity at the level
of the entire school, whereas external factors such as prey concentration and temperature are merely secondary drivers. 相似文献
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Previous studies point out a large (untapped) potential for energy efficiency in industry through the adoption of energy management practices. The aim of this paper is to describe and analyze energy management practices in two different Swedish energy-intensive industries: the pulp and paper industry and the foundry industry. The results show that one third of the studied mills and about two fifths of the studied foundries do not allocate energy costs by means of sub-metering, which probably contributes to reinforce the split incentive problem. Moreover, about one fifth of the mills and about half of the foundries lack a long-term energy strategy. The results also show that only about 40% and 25% respectively of the studied mills and foundries may be categorized as successful when it comes to energy management practices. If energy management is not fully prioritized even in energy-intensive industries – such as the studied foundry and pulp- and paper industry it will, in all probability, not be prioritized in less energy-intensive industrial sectors or countries either, indicating a large untapped potential in regard to cleaner, more environmentally sound, production in the industrial sector. 相似文献
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Water concentrations of PCDD/Fs, HCB, and non-ortho, mono-ortho, and non-dioxin-like PCBs were measured four times during 1 year in a coastal area of the Baltic Sea, to investigate background levels and distribution behaviour. Sampling sites included two rivers, an estuary, and the sea. Particulate and apparently dissolved concentrations were determined using active sampling (filters + PUFs), while freely dissolved concentrations were determined using passive sampling (POM-samplers). The distribution between particulate + colloidal and freely dissolved phases, in the form of TOC-normalized distribution ratios (KTOC), was found to be near or at equilibrium. The observed KTOC were not significantly different between sampling sites or seasons. For PCDD/Fs, the concentrations were significantly correlated to suspended particulate matter (SPM), while no correlation to organic carbon (TOC) was observed. In the estuary and the sea, PCB concentrations were correlated to TOC. The sorption of various congeners to SPM and TOC appeared to be related to both hydrophobicity and 3D-structure. The PCDD/F concentration in the sea decreased to one third in May, likely connected to the increased vertical flux of particles during the spring bloom. 相似文献
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The processes governing distribution of a xenobiotic compound discharged initially into the environment are discussed, and attention is drawn to (a) binding to organic matter in the sediment phase which affects both persistence and toxicity to biota and (b) the role of atmospheric transport for compounds of low water solubility and high vapour pressure. Important limitations in the use of sum parameters such as EOCI are pointed out. The important distinction between biodegradation and biotransformation is pointed out, and significant experimental determinants noted. Pathways for the aerobic metabolism of chlorophenolic compounds are discussed, and attention is drawn to the role of O‐methylation as an environmentally significant alternative to biodegradation. Evidence for the biodegradation of chlorinated aliphatic acids and hydrocarbons under both aerobic and anaerobic conditions is presented. Anaerobic metabolism of chlorophenolic compounds is discussed with respect to (a) de‐O‐methylation of chloroguaiacols, (b) dechlorination of chlorocatechols and (c) reduction of chlorovanillins. It is emphasized that current evidence provides a complex metabolic picture, and that only partial dechlorination may occur. Brief attention is given to the important issue of the persistence of chlorolignin, and attention drawn to technical issues which render this problem difficult of access by traditional procedures. Biohalogenation—particularly by fungi—is noted, though its quantitative contribution cannot be estimated at the moment. A number of important unresolved issues are underscored: (a) the problem of determining rates of microbial reactions which may be translated to environmental situations, (b) the cardinal role not only of the number of chlorine atoms in an aromatic compound but also the substitution pattern and (c) limitations in current understanding of the role of anaerobic bacteria in bringing about biodegradation and biotransformation. 相似文献